For his YouTube channel Listening In, Barnaby Martin analyzed the theme that Radiohead wrote for the 2015 Bond film Spectre, a song that he calls "one of the greatest Bond themes ever written". Somewhat notoriously (at least around these parts), the producers rejected this theme in favor of a lukewarm by Sam Smith.
After watching Martin's video, you should watch the Spectre opening credits sequence with the Radiohead theme — it's so much better than the theme they used in the film.